January 2008, to be published in Physical Review B1


Magnetic-polaron-driven magnetoresistance in the pyrochlore Lu$_{2}$V$_{2}$O$_{7}$
H. D. Zhou, E. S. Choi, J. A. Souza, J. Lu, Y. Xin, L. L. Lumata, B. S. Conner, L. Balicas, J. S. Brooks, J. J. Neumeier, and C. R. Wiebe

The structural, magnetic, and transport properties of single crystalline Lu$_{2}$V$_{2}$O$_{7}$ are studied. Lu$_{2}$V$_{2}$O$_{7}$ shows a ferromagnetic transition at \Tc~= 69.5 K and a negative magnetoresistance (MR) as high as 50 percent at \TS~= 75 K with an applied field of 5 T. Through various experiments, it is demonstrated that the mechanism for the MR is not through double-exchange, but through a polaron mediated behavior similar to Tl$_{2}$Mn$_{2}$O$_{7}$. This places Lu$_{2}$V$_{2}$O$_{7}$ as the only other example of polaron mediated MR among the pyrochlore oxides.

© 2008 The American Physical Society.